You Get The Leary You Deserve

The Leary Project

(Audio)
Beyond Life with Timothy Leary
11 mp3s - Beyond Life with Timothy Leary is a bit of a bizarre release. A combination of interviews, new music that ranges from ambient dance to Ministry and excerpts from Leary's 1967 album Turn On, Tune In Drop Out, the record attempts to create a trance-like atmosphere, one perfect for his vaguely mystical new age sentiments. - AMG
Turn On, Tune In, Drop Out (OMPS)
4 mp3s - Timothy Leary, PhD., Speaks on L.S.D. Leary’s rarest LP is also one of his best. Recorded at Millbrook and all spoken word.
Space Ghost interview (mp3)

(Video)
Timothy Leary's Last Trip
This authorized documentary of Leary's life pays homage to Leary and other '60s counterculture personalities such as Ken Kesey and the Merry Pranksters... - Rotten Tomatoes
Getting High - The History of LSD
An episode of The History Channel's History's Mysteries series
LSD - The Beyond Within part 1 part 2
1986 BBC documentary

As well as letters, a ridiculous amount of photos, and more.

I posted this a while back on MetaFilter (mining the archives!), and sure enough the thread is bright full of additional fun Leary/LSD linkage and commentary.